Synthesis and structures of palladium(II) and platinum(II) complexes containing heterocyclic thiolate ligands formed by cycloaddition reactions of coordinated azides

Author(s)
Angela Fleischer, Alexander Roller, Vladimir Arion, Bernhard Keppler, Fabian Mohr
Abstract

The phosphine-stabilized azido complexes [M(N3) 2(PTA)2] (M = Pd, Pt; PTA = 1,3,5-triaza-7- phosphaadamantane) were prepared in high yields by a ligand exchange reaction from cis-[Pd(N3)2(tmeda)] and cis-[Pt(N3) 2(cod)], respectively. The Pd and Pt complexes [M(N3) 2(PTA)2] undergo cycloaddition reactions with various isothiocyanates to give complexes containing anionic, S-coordinated tetrazole-thiolate ligands of the type trans-[M(SCN4R) 2(PTA)2] (M = Pd, Pt; R = Et, allyl, Me, Ph). The molecular structures of several of these derivatives were determined by X-ray crystallography.

Organisation(s)
Department of Inorganic Chemistry
External organisation(s)
Bergische Universität Wuppertal
Journal
Canadian Journal of Chemistry
Volume
87
Pages
146-150
No. of pages
5
ISSN
0008-4042
DOI
https://doi.org/10.1139/V08-115
Publication date
2009
Peer reviewed
Yes
Austrian Fields of Science 2012
104003 Inorganic chemistry
Portal url
https://ucrisportal.univie.ac.at/en/publications/73e67eda-9bae-4ac3-8efd-a0526f0a64ac