On the binding modes of metal NHC complexes with DNA secondary structures: Implications for therapy and imaging

Author(s)
Özden Karaca, Samuel M. Meier-Menches, Angela Casini, Fritz E. Kühn
Abstract

Organometallic compounds currently occupy an important place in the field of medicinal inorganic chemistry due to the unique chemical properties of metal coordination compounds. Particularly, metal compounds ligated by N-heterocyclic carbenes (NHC) have shown high potential for biomedical applications as antimicrobial and anticancer agents during the recent 15 years. Although further studies are necessary to validate the modes of action of this family of compounds, a number of biological targets have been identified, including DNA secondary structures. This perspective review aims at providing an overview of the most representative examples of metal NHC complexes reacting with nucleic acids via different binding modes. It is organized according to the type of DNA secondary structure targeted by metal NHCs, highlighting the possible advantages of biomedical applications, including therapy and imaging.

Organisation(s)
External organisation(s)
Technische Universität München, Cardiff University
Journal
Chemical Communications
Volume
53
Pages
8249-8260
No. of pages
12
ISSN
1359-7345
DOI
https://doi.org/10.1039/c7cc03074f
Publication date
2017
Peer reviewed
Yes
Austrian Fields of Science 2012
301303 Medical biochemistry, 104003 Inorganic chemistry, 301904 Cancer research
ASJC Scopus subject areas
Electronic, Optical and Magnetic Materials, Catalysis, Ceramics and Composites, General Chemistry, Surfaces, Coatings and Films, Metals and Alloys, Materials Chemistry
Sustainable Development Goals
SDG 3 - Good Health and Well-being
Portal url
https://ucrisportal.univie.ac.at/en/publications/9034fca7-d6a4-40f7-a8aa-cdcfeaae6849