Catalytically Active Gold Nanomaterials Stabilized by N-heterocyclic Carbenes

Author(s)
Constantin Eisen, Jia Min Chin, Michael R. Reithofer
Abstract

Solid supported or ligand capped gold nanomaterials (AuNMs) emerged as versatile and recyclable heterogeneous catalysts for a broad variety of conversions in the ongoing catalytic ' gold rush '. Existing at the border of homogeneous and heterogeneous catalysis, AuNMs offer the potential to merge high catalytic activity with significant substrate selectivity. Owing to their strong binding towards the surface atoms of AuMNs, NHCs offer tunable activation of surface atoms while maintaining selectivity and stability of the NM even under challenging conditions. This work summarizes well-defined catalytically active NHC capped AuNMs including spherical nanoparticles and atom-precise nanoclusters as well as the important NHC design choices towards activity and (stereo-)selectivity enhancements.

Organisation(s)
Department of Inorganic Chemistry, Department of Physical Chemistry
Journal
Chemistry: An Asian Journal
Volume
16
Pages
3026-3037
No. of pages
12
ISSN
1861-4728
DOI
https://doi.org/10.1002/asia.202100731
Publication date
08-2021
Peer reviewed
Yes
Austrian Fields of Science 2012
104003 Inorganic chemistry, 210004 Nanomaterials
Keywords
ASJC Scopus subject areas
Biochemistry, Organic Chemistry
Portal url
https://ucrisportal.univie.ac.at/en/publications/df411674-bf95-441b-8507-a1cea42abf5c