Isomerization pathway of a C–C sigma bond in a bis(octaazamacrocycle)dinickel(II) complex activated by deprotonation: a DFT study

Author(s)
Ingrid Jelemenska, Michal Zalibera, Peter Rapta, Anatolie Dobrov, Vladimir B. Arion, Lukas Bucinsky
Abstract

The anti (a) to syn (s) isomerization pathway of the deprotonated form of the dimer with two nickel(II) 15-membered octaazamacrocyclic units connected via a carbon–carbon (C–C) σ bond was investigated. For the initial anti (a) structure, a deprotonation of one of the bridging (sp3 hybridized) carbon atoms is suggested to allow for an a to s geometry twist. A 360° scan around the bridging C–C dihedral angle was performed first to find an intermediate geometry. Subsequently, the isomerization pathway was explored via individual steps using a series of mode redundant geometry optimizations (internal coordinates potential energy surface scans) and geometry relaxations leading to the s structure. The prominent geometries (intermediates) of the isomerization pathway are chosen and compared to the a and s structures, and geometry relaxations of the protonated forms of selected intermediates are considered.

Organisation(s)
Department of Inorganic Chemistry, Department of Biophysical Chemistry
External organisation(s)
Slovak University of Technology in Bratislava
Journal
Theoretical Chemistry Accounts
Volume
143
ISSN
1432-881X
DOI
https://doi.org/10.1007/s00214-024-03100-5
Publication date
04-2024
Peer reviewed
Yes
Austrian Fields of Science 2012
104022 Theoretical chemistry, 104017 Physical chemistry
Keywords
ASJC Scopus subject areas
Physical and Theoretical Chemistry
Portal url
https://ucrisportal.univie.ac.at/en/publications/df444ea3-18d2-4cfa-97a8-7b93bacadb73