Bis- and Tris(carboxylato)platinum(IV) Complexes with Mixed Am(m)ine Ligands in the trans Position Exhibiting Exceptionally High Cytotoxicity

Author(s)
Bjoern R. Hoffmeister, Michaela Hejl, Michael A. Jakupec, Mathea Sophia Galanski, Bernhard K. Keppler
Abstract

A series of seven diam(m)inebis(carboxylato)dihydroxidoplatinum(IV) and eleven diam(m)inetris(carboxylato)hydroxidoplatinum(IV) complexes with am(m)ine ligands in the trans position was synthesized and characterized by multinuclear

1H,

13C,

15N,

195Pt NMR spectroscopy. IC

50 values for all eighteen substances were determined by means of the 3-(4,5-dimethylthiazol-2-yl)-2,5-diphenyl-2H-tetrazolium bromide (MTT) assay for three human cancer cell lines. In cisplatin-sensitive CH1(PA-1) cancer cells, diam(m)inebis(carboxylato)dihydroxidoplatinum(IV) complexes displayed 50 % inhibitory concentrations in the micromolar range, whereas for the most lipophilic compounds of the diam(m)inetris(carboxylato)hydroxidoplatinum(IV) series, promising IC

50 values in the nanomolar range were found.

Organisation(s)
Department of Inorganic Chemistry, NMR Centre
Journal
European Journal of Inorganic Chemistry
Volume
2015
Pages
1700-1708
No. of pages
9
ISSN
1434-1948
DOI
https://doi.org/10.1002/ejic.201403226
Publication date
04-2015
Peer reviewed
Yes
Austrian Fields of Science 2012
104003 Inorganic chemistry, 301904 Cancer research
Keywords
ASJC Scopus subject areas
Inorganic Chemistry
Sustainable Development Goals
SDG 3 - Good Health and Well-being
Portal url
https://ucrisportal.univie.ac.at/en/publications/f14d477f-c165-4c18-b2e5-64bd38337f21